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Utilizing Lubricant Loss from Omniphobic Coatings as a Multifunctional Delivery Mechanism AITranslate

Karolinska Institutet Ming Wai Lau Centre for Reparative Medicine; City University of Hong Kong;Karolinska Institutet Ming Wai Lau Centre for Reparative Medicine;Karolinska Institutet Ming Wai Lau Centre for Reparative Medicine;Karolinska Institutet Ming Wai Lau Centre for Reparative Medicine; The Chinese University of Hong Kong; City University of Hong Kong;Karolinska Institutet Ming Wai Lau Centre for Reparative Medicine
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Publisher: ACS
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Abstract AITranslate

Silicon-based lubricant-infused surfaces (LIS) have revolutionized the surface and interface science field with their omniphobic properties. Polydimethylsiloxane (PDMS) LIS have demonstrated excellent potential for many biological, food, or cosmetic applications. However, translation into industry faces limitations for synthesis methodologies, reagent expense, retention of omniphobicity, and legislature concerning lubricant migration. Preventing lubricant loss and retention of omniphobicity has been widely investigated, but what if the gradual lubricant depletion could be utilized for releasing active agents? Herein, we produce silicone-based organogel LIS via spontaneous 1-step polyurea reactions (Silgels) and functionalize with silver nanoparticles (Ag NP). We comparatively examined their physicochemical properties, omniphobic dewetting for probe liquids and complex mixtures (foodstuffs), and biocompatibility with mammalian and bacterial cultures. Overall, we present an easily scalable methodology to produce multifunctional, biocompatible LIS that has potential for the food packaging, cosmetic, and biological industries.

KeyWords AITranslate

omniphobic polydimethylsiloxane lubricant infused surfaces (LIS) silver nanoparticles organogel
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Basic Information:

DOI:https://doi.org/10.1021/acsapm.2c01991

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Citation Information:

Silicon-based lubricant-infused surfaces (LIS) have revolutionized the surface and interface science field with their omniphobic properties. Polydimethylsiloxane (PDMS) LIS have demonstrated excellent potential for many biological, food, or cosmetic applications. However, translation into industry faces limitations for synthesis methodologies, reagent expense, retention of omniphobicity, and legislature concerning lubricant migration. Preventing lubricant loss and retention of omniphobicity has been widely investigated, but what if the gradual lubricant depletion could be utilized for releasing active agents? Herein, we produce silicone-based organogel LIS via spontaneous 1-step polyurea reactions (Silgels) and functionalize with silver nanoparticles (Ag NP). We comparatively examined their physicochemical properties, omniphobic dewetting for probe liquids and complex mixtures (foodstuffs), and biocompatibility with mammalian and bacterial cultures. Overall, we present an easily scalable methodology to produce multifunctional, biocompatible LIS that has potential for the food packaging, cosmetic, and biological industries.

quote

GB/T 7714-2015 [1] Callum Stewart, Babak Mehrjou, Hui Huang, et al. ACS Applied Polymer Materials, 2023(5). DOI:10.1021/acsapm.2c01991.
MLA [1] Callum Stewart, et al., ACS Applied Polymer Materials, no. 5, 2023, https://doi.org/10.1021/acsapm.2c01991.
APA [1] Callum Stewart, Babak Mehrjou, Hui Huang, Yunxin Long, Kyler Chow, Tsz Wai Kok, Paul K. Chu, & Linxian Li. (2023). ACS Applied Polymer Materials(5). https://doi.org/10.1021/acsapm.2c01991
IEEE [1] Callum Stewart, Babak Mehrjou, Hui Huang, Yunxin Long, Kyler Chow, Tsz Wai Kok, Paul K. Chu, and Linxian Li, ACS Applied Polymer Materials, no. 5, 2023, doi: 10.1021/acsapm.2c01991. keywords: {omniphobic;polydimethylsiloxane;lubricant infused surfaces (LIS);silver nanoparticles;organogel}