Study on Ultrasonic-Microwave Synergistic Oxidation Leaching of Tellurium from Copper-separated Residue of Copper Anode Slime Based on RSM AITranslate
Abstract AITranslate
In alkaline system,the method of ultrasonic-microwave synergistic oxidation leaching with the oxidant of NaClO3 was used to extract tellurium from copper-separated residue of copper anode slime.Based on the model optimal design principle of response surface method,the multiple quadratic regression equation of the influence of ultrasonic power,microwave power,reaction time and their interaction on the tellurium leaching rate was established,and the optimal leaching process was obtained.The results show that the optimal conditions of ultrasonic leaching are ultrasonic power 150 W,ultrasonic time 30 min,leaching temperature 90 ℃,NaClO3 addition amount 1.5 times copper-separated residue amount,liquid-solid ratio 9∶1 and NaOH concentration 1.2 mol/L,and the leaching rate of tellurium reaches 93.15%.The optimal conditions of microwave leaching are microwave power 700 W,microwave time 4 min,liquid-solid ratio 10∶1,temperature 85 ℃ and NaClO3 addition amount 1.2 times copper-separated residue amount,and the leaching rate of tellurium reaches 91.08%.The optimal conditions of ultrasonic-microwave leaching are ultrasonic power 414 W,microwave power 287 W and reaction time 14 min,and the predicted leaching rate of tellurium is 96.73%.The model is a second-order polynomial model.Compared with the average leaching rate of 93.40%±0.95% obtained in the validation experiment,the predicted value has little deviation,which is consistent with the model.
KeyWords AITranslate
1闫晓淼,李先如,卫皇曌,何松波,余丽,孙承林.响应面法在催化湿式氧化降解异佛尔酮中的应用[J].环境化学,2012,31(12):1865-1873. 被引量：3
2李长龙,彭金辉,张利波,李雨,雷鹰,段昕辉.响应曲面法优化硫酸铵微波干燥工艺[J].化学工程,2011,39(3):8-12. 被引量：7
3章尚发,王冲,王华,杨坤彬,李英伟.氯化浸出-还原法处理铜阳极泥分铜渣[J].稀有金属与硬质合金,2014,42(1):5-8. 被引量：11
4马致远,杨洪英.响应曲面法优化铜阳极泥微波浸出硒工艺[J].中南大学学报：自然科学版,2015,46(7):2391-2397. 被引量：26
5廖亚龙,周娟,黄斐荣,王祎洋.响应曲面法优化复杂硫化铜矿选择性浸出工艺[J].中国有色金属学报,2016,26(1):164-172. 被引量：15
6彭万金.超声波在冶金中的应用研究[J].上海有色金属,2008,29(3):135-139. 被引量：8
7陈安安,周少奇,赵晶晶.镍铁尾矿酸浸过程的响应曲面分析[J].现代化工,2013,33(2):99-103. 被引量：4
8刘伟锋,杨天足,刘又年,陈霖,张杜超,王安.脱除铜阳极泥中贱金属的预处理工艺[J].中南大学学报：自然科学版,2013,44(4):1332-1337. 被引量：22
9R.Palanivel,P.Koshy Mathews.Prediction and optimization of process parameter of friction stir welded AA5083-H111 aluminum alloy using response surface methodology[J].中南大学学报：英文版,2012,19(1):1-8. 被引量：26
10袁武华,王峰.国内外易切削钢的研究现状和前景[J].钢铁研究,2008,36(5):56-62. 被引量：52
1廖春发,邹耕,彭珊,邹建柏,周迅.从铜阳极泥分铜渣碱浸液中回收碲[J].湿法冶金,2021,40(2):120-124. 被引量：2
2赵刘闯,赵建章,周立云,李少平,江旭,王露露.贵州某金矿浮选条件的响应曲面法优化研究[J].贵金属,2021,42(3):58-63. 被引量：1
3程明宇,潘高,黄义威,赵伟康,于明明,梅光军.微波辅助盐酸浸出废弃荧光粉中的稀土元素钇和铕[J].金属矿山,2022(5):153-159.
4曾颜亮,彭珊,廖春发,刘付朋.水浸分铜渣超声波外场强化碱浸分碲动力学研究[J].稀有金属与硬质合金,2023,51(3):30-36. 被引量：1
1喻小强,徐家聪,易勤,温盛汇,田磊.高砷铅阳极泥常压碱浸脱砷试验研究[J].湿法冶金,2021,40(4):342-346. 被引量：4
2黄海飞,欧阳谦涛,崔胜,彭昭成,张圣南,杨跃新.50t/a湿法提碲生产线工艺设计与生产实践[J].湖南有色金属,2022,38(6):25-28.
3许才武,蒋中刚,唐道文,袁鑫,邹涛,邱洋.响应曲面法优化NaClO浸出贵州难浸金矿中的金[J].贵金属,2023,44(2):62-68.
4曾颜亮,邹建柏,廖春发,刘付朋.SO_(2)还原SeO_(2)制备Se的工艺及动力学研究[J].稀有金属与硬质合金,2023,51(4):33-38.
1杜欣,王天泽,陈渡文,于景成,沙广燕.基于绿色化学理念的苯甲醛与安息香的相互转化[J].大学化学,2020,35(4):19-26. 被引量：5
2朱若非,林佳琦,宋少飞.铅冶炼厂还原炉烟灰中铅锌超声波浸出分离试验[J].黄金,2019,40(2):73-76.
3朱兴彩,杨坤.超声波强化低品位氧化锌矿在NH_3-(NH_4)_2SO_4-H_2O体系中的浸出[J].矿冶,2018,27(1):37-40. 被引量：3
4曹雪娇,张廷安,刘燕,张伟光,李思敏,吕国志,韩秀秀.臭氧强化氧化氧化锌法脱硫过程中产生的亚硫酸锌[J].有色金属科学与工程,2020,11(1):1-7. 被引量：2
5王琴,罗洁莹,柳建良,刘袆帆.响应面法优化超声-微波协同辅助提取金柚幼果总黄酮工艺[J].食品研究与开发,2020,41(2):83-91. 被引量：12
6万青珂,张洋,郑诗礼,张盈,王晓健,娄文博,JAN J.Weigand,MARCO Wenzel.废旧磷酸铁锂正极粉磷酸浸出过程的优化及宏观动力学[J].化工进展,2020,39(6):2495-2502. 被引量：7
7沈文龙,宋镇,张波,谢铭露,乔璐,朱冰.杏鲍菇热泵干燥特性及工艺参数优化[J].中国农机化学报,2019,40(10):135-141. 被引量：9
8刘淑婷,王颖,王志辉,王迪,张艳莉.超声-微波协同酶法制备芸豆抗性淀粉工艺优化及结构分析[J].中国食品学报,2020,20(5):187-195. 被引量：11
9刘二燕,薛飞,许士洪,李登新.微波与酶联用对印染污泥脱水性能的影响[J].环境工程,2020,38(5):13-17. 被引量：2
10李强,杨皓迪,李奇勇,黄舒宁,邢丹霞.湿法炼锌净化钴渣酸浸液萃取除杂试验研究[J].湿法冶金,2020,39(2):151-155. 被引量：6
Basic Information:
DOI：
Chinese Library Classification Number:TF803.2[冶金工程—有色金属冶金]
Citation Information:
In alkaline system,the method of ultrasonic-microwave synergistic oxidation leaching with the oxidant of NaClO3 was used to extract tellurium from copper-separated residue of copper anode slime.Based on the model optimal design principle of response surface method,the multiple quadratic regression equation of the influence of ultrasonic power,microwave power,reaction time and their interaction on the tellurium leaching rate was established,and the optimal leaching process was obtained.The results show that the optimal conditions of ultrasonic leaching are ultrasonic power 150 W,ultrasonic time 30 min,leaching temperature 90 ℃,NaClO3 addition amount 1.5 times copper-separated residue amount,liquid-solid ratio 9∶1 and NaOH concentration 1.2 mol/L,and the leaching rate of tellurium reaches 93.15%.The optimal conditions of microwave leaching are microwave power 700 W,microwave time 4 min,liquid-solid ratio 10∶1,temperature 85 ℃ and NaClO3 addition amount 1.2 times copper-separated residue amount,and the leaching rate of tellurium reaches 91.08%.The optimal conditions of ultrasonic-microwave leaching are ultrasonic power 414 W,microwave power 287 W and reaction time 14 min,and the predicted leaching rate of tellurium is 96.73%.The model is a second-order polynomial model.Compared with the average leaching rate of 93.40%±0.95% obtained in the validation experiment,the predicted value has little deviation,which is consistent with the model.
quote
| GB/T 7714-2015 | [1] LIAO Chun-fa, PENG Shan, ZOU Geng, et al. Study on Ultrasonic-Microwave Synergistic Oxidation Leaching of Tellurium from Copper-separated Residue of Copper Anode Slime Based on RSM[J]. Rare Metals and Cemented Carbides, 2020(2): 10-17. |
| MLA | [1] LIAO Chun-fa, et al., "Study on Ultrasonic-Microwave Synergistic Oxidation Leaching of Tellurium from Copper-separated Residue of Copper Anode Slime Based on RSM." Rare Metals and Cemented Carbides, no. 2, 2020, pp. 10-17. |
| APA | [1] LIAO Chun-fa, PENG Shan, ZOU Geng, & ZENG Yan-liang. (2020). Study on Ultrasonic-Microwave Synergistic Oxidation Leaching of Tellurium from Copper-separated Residue of Copper Anode Slime Based on RSM. Rare Metals and Cemented Carbides(2), 10-17. |
| IEEE | [1] LIAO Chun-fa, PENG Shan, ZOU Geng, and ZENG Yan-liang, "Study on Ultrasonic-Microwave Synergistic Oxidation Leaching of Tellurium from Copper-separated Residue of Copper Anode Slime Based on RSM," Rare Metals and Cemented Carbides, no. 2, pp. 10-17, 2020. keywords: {copper-separated residue;tellurium;ultrasonic;microwave;oxidation leaching;RSM} |