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Ultraviolet-Induced Gas Sensing Performance of Ag/WO3/rGO Nanocomposites for H2S Gas Sensors Ultraviolet-Induced Gas Sensing Performance of Ag/WO3/rGO Nanocomposites for H2S Gas Sensors AITranslate

Zhengzhou University of Light Industry; Zhengzhou University of Light Industry; Zhengzhou University of Light Industry; Zhengzhou University of Light Industry; Zhengzhou University of Light Industry; Zhengzhou University of Light Industry; Hubei Institute of Aerospace Chemotechnology; Hubei Institute of Aerospace Chemotechnology; Huazhong University of Science and Technology
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Publisher: ACS
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Abstract AITranslate

The attention toward cost-effective and high-performance H2S sensors is increasing due to the growing need for physical health and environmental monitoring. In this paper, Ag/WO3/reduced graphene oxide (rGO) nanocomposites were synthesized by using a microwave-assisted gas–liquid interfacial method. Nanomaterials with different Ag doping contents were successfully prepared with AgNO3 as an additive. The Ag/WO3/rGO sensors exhibit remarkable selectivity toward H2S, and the gas sensing performances of Ag-doped WO3/rGO gas sensors are significantly better than those of WO3/rGO. At 150 °C, the response value of the 10 wt % Ag/WO3/rGO gas sensor to 100 ppm H2S is 204.5, which is 7 times higher than that of WO3/rGO, and the response/recovery time of the sensor is 9/49 s, respectively. Additionally, the gas sensing performance of the sensor is further enhanced under ultraviolet (UV) irradiation. The response value is enhanced to 685.8, which is 3 times higher than that without UV irradiation, and the response/recovery time is reduced to 8/38 s, respectively. The sensing mechanism is also discussed. This work offers a potential application for H2S detection in environmental monitoring and smart healthcare.

KeyWords AITranslate

WO3/rGO Ag doping H2S gas sensor ultravioletinduced gas−liquid interfacial
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Basic Information:

DOI:https://doi.org/10.1021/acsaelm.3c00349

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Citation Information:

The attention toward cost-effective and high-performance H2S sensors is increasing due to the growing need for physical health and environmental monitoring. In this paper, Ag/WO3/reduced graphene oxide (rGO) nanocomposites were synthesized by using a microwave-assisted gas–liquid interfacial method. Nanomaterials with different Ag doping contents were successfully prepared with AgNO3 as an additive. The Ag/WO3/rGO sensors exhibit remarkable selectivity toward H2S, and the gas sensing performances of Ag-doped WO3/rGO gas sensors are significantly better than those of WO3/rGO. At 150 °C, the response value of the 10 wt % Ag/WO3/rGO gas sensor to 100 ppm H2S is 204.5, which is 7 times higher than that of WO3/rGO, and the response/recovery time of the sensor is 9/49 s, respectively. Additionally, the gas sensing performance of the sensor is further enhanced under ultraviolet (UV) irradiation. The response value is enhanced to 685.8, which is 3 times higher than that without UV irradiation, and the response/recovery time is reduced to 8/38 s, respectively. The sensing mechanism is also discussed. This work offers a potential application for H2S detection in environmental monitoring and smart healthcare.

quote

GB/T 7714-2015 [1] Yanghai Gui, Jintao Wu, Kuan Tian, et al. ACS Applied Electronic Materials, 2023(5). DOI:10.1021/acsaelm.3c00349.
MLA [1] Yanghai Gui, et al., ACS Applied Electronic Materials, no. 5, 2023, https://doi.org/10.1021/acsaelm.3c00349.
APA [1] Yanghai Gui, Jintao Wu, Kuan Tian, Huishi Guo, Xiaoyun Qin, Xiaomei Qin, Xiang Guo, Canxiang Fang, & Peng Liu. (2023). ACS Applied Electronic Materials(5). https://doi.org/10.1021/acsaelm.3c00349
IEEE [1] Yanghai Gui, Jintao Wu, Kuan Tian, Huishi Guo, Xiaoyun Qin, Xiaomei Qin, Xiang Guo, Canxiang Fang, and Peng Liu, ACS Applied Electronic Materials, no. 5, 2023, doi: 10.1021/acsaelm.3c00349. keywords: {WO3/rGO Ag doping H2S gas sensor ultravioletinduced gas−liquid interfacial}