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A Biomimetic Water-Resistant Adhesive Based on ε-Polylysine/Tannic Acid Complexation AITranslate

Technical University of Denmark; Technical University of Denmark; Technical University of Denmark; Technical University of Denmark
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Publisher: ACS
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Abstract AITranslate

This study investigates the potential of combining ε-polylysine and tannic acid to develop bio-based adhesives with enhanced water resistance. The two biomolecules exhibited complexation/precipitation in aqueous solutions in the pH range of 5–9. Water-based adhesives were prepared using complexes formed at pH 5, 7, and 9, followed by evaluation of their adhesion properties in both dry and wet lap shear tests. The complexes prepared at higher pH values showed a larger adhesion strength and improved water resistance. To further enhance the adhesive properties, an epoxide-based reagent was utilized to double-cross-link the complexes, resulting in a lap shear strength of ∼2 MPa after being submerged in water for 7 days.

KeyWords AITranslate

biobased adhesive water resistance polylysine tannic acid marineinspired adhesive
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Basic Information:

DOI:https://doi.org/10.1021/acsapm.3c01400

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Citation Information:

This study investigates the potential of combining ε-polylysine and tannic acid to develop bio-based adhesives with enhanced water resistance. The two biomolecules exhibited complexation/precipitation in aqueous solutions in the pH range of 5–9. Water-based adhesives were prepared using complexes formed at pH 5, 7, and 9, followed by evaluation of their adhesion properties in both dry and wet lap shear tests. The complexes prepared at higher pH values showed a larger adhesion strength and improved water resistance. To further enhance the adhesive properties, an epoxide-based reagent was utilized to double-cross-link the complexes, resulting in a lap shear strength of ∼2 MPa after being submerged in water for 7 days.

quote

GB/T 7714-2015 [1] Junjie Kang, Saeed Zajforoushan Moghaddam, René Wugt Larsen, et al. ACS Applied Polymer Materials, 2023(5). DOI:10.1021/acsapm.3c01400.
MLA [1] Junjie Kang, et al., ACS Applied Polymer Materials, no. 5, 2023, https://doi.org/10.1021/acsapm.3c01400.
APA [1] Junjie Kang, Saeed Zajforoushan Moghaddam, René Wugt Larsen, & Esben Thormann. (2023). ACS Applied Polymer Materials(5). https://doi.org/10.1021/acsapm.3c01400
IEEE [1] Junjie Kang, Saeed Zajforoushan Moghaddam, René Wugt Larsen, and Esben Thormann, ACS Applied Polymer Materials, no. 5, 2023, doi: 10.1021/acsapm.3c01400. keywords: {biobased adhesive;water resistance;polylysine;tannic acid;marineinspired adhesive}