daohang fenxiangbox searchbox qikanlogonew daohangnew searchboxnew navrightzone footerzone paper
English
Chinese 简体中文 English English
Home > Journals > ACS Applied Electronic Materials
‹ Previous Article Next Article ›

Magnetic Anisotropy and Jahn–Teller Effect in Ferromagnetic Two-Dimensional CrGa2Te4 Magnetic Anisotropy and Jahn–Teller Effect in Ferromagnetic Two-Dimensional CrGa2Te4 AITranslate

Chenghuan Jiang; Kangjun Lu; Ruqian Wang; Qian Chen; Jinlan Wang
Nanjing Institute of Technology; Southeast University; Southeast University; Southeast University; Southeast University
AITranslate
Publisher: ACS
Share Citation Information Add to Favorites

    Scan to share on WeChat or Moments

Use WeChat scan.
Share with WeChat friends or Moments

Abstract AITranslate

The transition metal (TM)-based two-dimensional (2D) materials show great promise for realizing ultrathin spintronic devices because of their structural and magnetic properties. In this work, we predict the ferromagnetic ground state of the CrGa2Te4 monolayer with an α-FeGa2S4-1T type phase. The first-principles calculations and Monte Carlo simulations indicate that this monolayer is a ferromagnetic half-metal possessing a Curie temperature of 277 K. It is revealed in this system that the further splitting of Cr-eg orbitals results in a high-spin configuration of Cr2+ with an out-of-plane easy axis. A physical picture of the magneto-crystalline anisotropy affected by the Jahn–Teller distortion in the GrCa2Te4 monolayer is obtained. This work expands our understanding of the magnetic phenomena to 2D octahedral coordinated crystals.

KeyWords AITranslate

twodimensional magnets magnetic anisotropy Curie temperatures spintronics density functional theory
No data

Basic Information:

DOI：https://doi.org/10.1021/acsaelm.2c00433

Chinese Library Classification Number:

Citation Information:

The transition metal (TM)-based two-dimensional (2D) materials show great promise for realizing ultrathin spintronic devices because of their structural and magnetic properties. In this work, we predict the ferromagnetic ground state of the CrGa2Te4 monolayer with an α-FeGa2S4-1T type phase. The first-principles calculations and Monte Carlo simulations indicate that this monolayer is a ferromagnetic half-metal possessing a Curie temperature of 277 K. It is revealed in this system that the further splitting of Cr-eg orbitals results in a high-spin configuration of Cr2+ with an out-of-plane easy axis. A physical picture of the magneto-crystalline anisotropy affected by the Jahn–Teller distortion in the GrCa2Te4 monolayer is obtained. This work expands our understanding of the magnetic phenomena to 2D octahedral coordinated crystals.

quote

GB/T 7714-2015 [1] Chenghuan Jiang, Kangjun Lu, Ruqian Wang, et al. ACS Applied Electronic Materials, 2022(4). DOI:10.1021/acsaelm.2c00433.
MLA [1] Chenghuan Jiang, et al., ACS Applied Electronic Materials, no. 4, 2022, https://doi.org/10.1021/acsaelm.2c00433.
APA [1] Chenghuan Jiang, Kangjun Lu, Ruqian Wang, Qian Chen, & Jinlan Wang. (2022). ACS Applied Electronic Materials(4). https://doi.org/10.1021/acsaelm.2c00433
IEEE [1] Chenghuan Jiang, Kangjun Lu, Ruqian Wang, Qian Chen, and Jinlan Wang, ACS Applied Electronic Materials, no. 4, 2022, doi: 10.1021/acsaelm.2c00433. keywords: {twodimensional magnets magnetic anisotropy Curie temperatures spintronics density functional theory}