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Impact of the Microstructure on Electrochemical Performances of Dilithium Benzoquinone Dioximate as a Positive Material for a Li-Ion Battery AITranslate

Roberto Russo; Carine Davoisne; Adolfo Urrutia; Yann Danten; Carlo Gatti; Gwenaelle Toussaint; Philippe Stevens; Christine Frayret; Matthieu Becuwe
Université de Picardie Jules Verne; Université de Picardie Jules Verne; Université de Picardie Jules Verne;Institut des Sciences Moléculaires, UMR CNRS 5255;CNR SCITEC, CNR Istituto di Scienze e Tecnologie Chimiche “‘Giulio Natta”’;Department Electric Equipment Laboratory (LME);Department Electric Equipment Laboratory (LME); Université de Picardie Jules Verne; Université de Picardie Jules Verne
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Abstract AITranslate

Herein we would like to highlight the impact of the material microstructure on electrochemical performances of dilithium benzoquinone dioximate (Li2-BQDO) and its oxidized and self-polymerized version (PNND), a promising electroactive material for energy storage application. Li2-BQDO showed a reversible exchange of two lithium ions at high redox potential (3.0 V vs Li+/Li), acting as a lithiated organic positive electrode for lithium-ions batteries. After a preliminary computational study, electrochemical performance of the oxidized form of Li2-BQDO , which polymerize inside the cell, were also investigated. Thanks to TEM analysis coupled with the XRD experiment, the role of microstructure and crystal structure in the energy storage process was highlighted.

KeyWords AITranslate

Organic batteries positive electrode dioximate selfpolymerization Transmission Electron Microscopy benzoquinone dioxime Show More
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Basic Information:

DOI：https://doi.org/10.1021/acsapm.3c01618

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Citation Information:

Herein we would like to highlight the impact of the material microstructure on electrochemical performances of dilithium benzoquinone dioximate (Li2-BQDO) and its oxidized and self-polymerized version (PNND), a promising electroactive material for energy storage application. Li2-BQDO showed a reversible exchange of two lithium ions at high redox potential (3.0 V vs Li+/Li), acting as a lithiated organic positive electrode for lithium-ions batteries. After a preliminary computational study, electrochemical performance of the oxidized form of Li2-BQDO , which polymerize inside the cell, were also investigated. Thanks to TEM analysis coupled with the XRD experiment, the role of microstructure and crystal structure in the energy storage process was highlighted.

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GB/T 7714-2015 [1] Roberto Russo, Carine Davoisne, Adolfo Urrutia, et al. ACS Applied Polymer Materials, 2023(5). DOI:10.1021/acsapm.3c01618.
MLA [1] Roberto Russo, et al., ACS Applied Polymer Materials, no. 5, 2023, https://doi.org/10.1021/acsapm.3c01618.
APA [1] Roberto Russo, Carine Davoisne, Adolfo Urrutia, Yann Danten, Carlo Gatti, Gwenaelle Toussaint, Philippe Stevens, Christine Frayret, & Matthieu Becuwe. (2023). ACS Applied Polymer Materials(5). https://doi.org/10.1021/acsapm.3c01618
IEEE [1] Roberto Russo, Carine Davoisne, Adolfo Urrutia, Yann Danten, Carlo Gatti, Gwenaelle Toussaint, Philippe Stevens, Christine Frayret, and Matthieu Becuwe, ACS Applied Polymer Materials, no. 5, 2023, doi: 10.1021/acsapm.3c01618. keywords: {Organic batteries;positive electrode;dioximate;selfpolymerization;Transmission Electron Microscopy;benzoquinone dioxime;Show More}