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Engineering Stable Perovskite Film for High Color Purity Display Application AITranslate

Friedrich-Alexander-Universität Erlangen-Nürnberg, Materials for Electronics and Energy Technology (i-MEET);Friedrich-Alexander-Universität Erlangen-Nürnberg, Materials for Electronics and Energy Technology (i-MEET);Friedrich-Alexander-Universität Erlangen-Nürnberg, Materials for Electronics and Energy Technology (i-MEET);Friedrich-Alexander-Universität Erlangen-Nürnberg, Materials for Electronics and Energy Technology (i-MEET);Friedrich-Alexander-Universität Erlangen-Nürnberg, Materials for Electronics and Energy Technology (i-MEET);Friedrich-Alexander-Universität Erlangen-Nürnberg, Materials for Electronics and Energy Technology (i-MEET)
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Publisher: ACS
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Abstract AITranslate

Lead halide perovskite nanocrystals (NCs) are the most promising candidates for displays satisfying the Rec. 2020 UHDTV color standard. However, moisture sensitivity currently limits light-emitting applications requiring color stability and purity. In this study, we propose a large-area FAPbBr3-based quantum dot brightness enhancing film (QDEF) strategy developed in our group five years ago. The combination of a polymeric binder tailored to the ligands optimized perovskite NCs for light conversion and demonstrates QDEF applications with 91% coverage of Rec. 2020 standard in tablet displays, using polyhedral oligomeric silsesquioxane-capped FAPbBr3 as the green emitter and K2SiF6: Mn4+ (KSF) as a red emitter. Remarkably, our films operating in displays showed 4 year stability without lead leakage. Even without barrier protection, the unpackaged QDEF maintained 55% of its initial performance. This highlights the importance of a dual stabilization strategy for extending operational and shelf lifetimes of advanced functional perovskite composites.

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DOI:https://doi.org/10.1021/acsenergylett.3c01812

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Citation Information:

Lead halide perovskite nanocrystals (NCs) are the most promising candidates for displays satisfying the Rec. 2020 UHDTV color standard. However, moisture sensitivity currently limits light-emitting applications requiring color stability and purity. In this study, we propose a large-area FAPbBr3-based quantum dot brightness enhancing film (QDEF) strategy developed in our group five years ago. The combination of a polymeric binder tailored to the ligands optimized perovskite NCs for light conversion and demonstrates QDEF applications with 91% coverage of Rec. 2020 standard in tablet displays, using polyhedral oligomeric silsesquioxane-capped FAPbBr3 as the green emitter and K2SiF6: Mn4+ (KSF) as a red emitter. Remarkably, our films operating in displays showed 4 year stability without lead leakage. Even without barrier protection, the unpackaged QDEF maintained 55% of its initial performance. This highlights the importance of a dual stabilization strategy for extending operational and shelf lifetimes of advanced functional perovskite composites.

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GB/T 7714-2015 [1] Huiying Hu, Ievgen Levchuk, Felix Kalkowski, et al. ACS Energy Letters, 2023(8). DOI:10.1021/acsenergylett.3c01812.
MLA [1] Huiying Hu, et al., ACS Energy Letters, no. 8, 2023, https://doi.org/10.1021/acsenergylett.3c01812.
APA [1] Huiying Hu, Ievgen Levchuk, Felix Kalkowski, Jack Elia, Andres Osvet, & Christoph J. Brabec. (2023). ACS Energy Letters(8). https://doi.org/10.1021/acsenergylett.3c01812
IEEE [1] Huiying Hu, Ievgen Levchuk, Felix Kalkowski, Jack Elia, Andres Osvet, and Christoph J. Brabec, ACS Energy Letters, no. 8, 2023, doi: 10.1021/acsenergylett.3c01812.